I'm surprised we didn't have this discussion. I remembered the theme for The World Was Not Enough was dope. Trip Hop working really well with the bond theme. Also the singer from Garbage fits in so well. Lastly, that music video though wasn't a mainstay in my life, was really memorable from a maybe 7-8 year old me.
I don't have a personal favorite but my brother has two. He loves Tina Turner's theme from GoldenEye as well as Chris Cornell's "You Know My Name" from Casino Royale '06
In a similar fashion to that one is Sheryl Crow's Tomorrow never dies, which may be my favourite of the ones I've listened. I read it had bad reaction, well, each to their own... here it goes for you to judge by yourself:
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